Microscopic Understanding of Thermal-magnon Transport in a Low-damping Ferrimagnetic Thin Films

RESUMO

Thermally generated magnons enable heat-driven spin transport in magnetic insulators, yet the relative importance of multiple microscopic mechanisms governing their propagation remains incompletely understood. Here, we investigate thermal magnon transport in low-damping Li$_{0.5}$Al$_{1.0}$Fe$_{1.5}$O$_4$/Pt nanodevices using a nonlocal spin Seebeck geometry that separates magnon transport from local thermoelectric effects. Thermal imaging establishes a detector region outside the thermal healing length, enabling intrinsic nonlocal measurements. We find that thermal magnon transport is strongly suppressed by magnetic fields far above saturation, and further that thermal magnon transport decreases with increasing temperature despite an increasing magnon population. Brillouin light scattering reveals the key microscopic mechanism driving this effect: increasing field reduces the group velocity of backward volume magnons, directly reducing the magnon spin diffusion length. Micromagnetic simulations reproduce this behavior only when a temperature-dependent exchange stiffness is included. These results identify magnon group velocity and exchange stiffness as key parameters governing thermal magnon transport in ferrimagnetic thin films.