Breathers in solitonic room-temperature superlattice-induced superfluorescence in quasi-2D perovskites

RESUMO

Recently, a soliton mechanism for room-temperature superfluorescence in thin perovskite films has been proposed, with a fundamental soliton predicted to remain stable under LO phonon--exciton interactions. At the same time, superlattice architectures offer a route to enhancing superfluorescence in perovskites. Motivated by recent observations of room-temperature superfluorescence in periodic superlattices of quasi-2D metal-halide perovskites, we extend the 2D nonlocal nonlinear Schrödinger equation describing Wannier exciton--LO phonon interactions to superlattice structures, obtaining a 3D nonlocal nonlinear Schrödinger equation. We show that interlayer tunnelling gives rise to breather dynamics corresponding to a stable fundamental soliton in mixed coordinate--momentum space, with the coordinate parallel to the layers and the momentum perpendicular to them. The breather dynamics originate from miniband formation, which induces a momentum-dependent phase modulation of the soliton. In the absence of interlayer tunnelling, the breather dynamics disappear and the soliton becomes stationary. These results establish a direct connection between interlayer tunnelling, miniband formation and soliton dynamics, suggesting that breather behavior can provide a signature of interlayer tunnelling in quasi-2D perovskite superlattices.