Evidence of Crystal-Field-Mediated Anisotropic Orbital Rashba Effect in Epitaxial Ru/FM Heterostructure

RESUMO

Electrical generation of orbital angular momentum provides a promising route to current-induced torques, yet effective control of orbital Rashba textures still remains challenging, particularly because the role of the interfacial crystal field remains largely unexplored. Here, we report experimental evidence for a crystal-field-mediated interfacial anisotropic orbital Rashba effect (AORE) in epitaxial Ru/ferromagnet heterostructures. Total orbital torque was disentangled into an isotropic bulk contribution and an in-plane anisotropic interfacial contribution. The latter was strongly suppressed by degrading the crystallinity of either constituent and by inserting a Cu spacer, highlighting the essential roles of coherent interfacial orbital hybridization and direct Ru/ferromagnet contact. These results identify interfacial crystal-field coherency as a key ingredient in manipulating orbital Rashba textures and establish a route toward engineering the symmetry and directionality of orbital torques.